长江中下游六省大气甲烷柱浓度时空分布   总被引：2，自引：0，他引：2  

冯敏玉  张根  夏玲君  熊劦  李柏贞  孔萍  占明锦  张玉霞 《地球化学》2021,50(1):121-132

甲烷(CH4)是造成气候变暖的主要温室气体之一。为了了解长江中下游水稻种植区CH4浓度的分布情况,本次研究基于温室气体观测卫星(greenhouse gases observing satellite,GOSAT)和大气红外探测仪(atmospheric infrared sounder,AIRS)卫星反演的数据产品,对我国长江中下游六省大气CH4柱浓度的时空分布特征进行了研究。研究结果表明,由GOSAT反演的长江中下游六省大气CH4浓度呈逐年增长趋势,其年均浓度由2011年的1817×10^?9增长至2018年的1875×10^?9,高于东三省、华北平原和全国平均水平。区域平均年增长量为8.2×10^?9 a^?1。各省年际增长幅度略有差异,纬度偏低的江西、湖南和浙江三省大气CH4浓度高且增长量偏大,纬度偏高的湖北、安徽和江苏三省大气CH4浓度略低且增长量偏小。长江中下游六省大气CH4呈现较强的季节变化特征,湖北、湖南、江西和浙江峰值出现在9月,安徽、江苏峰值出现在8月。垂直方向上长江中下游六省CH4浓度随气压降低,浓度逐渐减小,呈现出明显的季节变化特征,近地面层GOSAT反演的最高值出现在夏季,最低值出现在春季;高层最高值出现在秋季,最低值出现在春季。AIRS反演的大气CH4浓度空间分布上北高南低,与GOSAT反演结果不一致,可能由于AIRS主要反映了对流层中层大气状况而GOSAT更多的反映了近地面层大气CH4的变化。其垂直方向上呈现高度越高,浓度越低,不同高度上秋季浓度均最高。  相似文献   

最近十多年来冰冻圈加速萎缩——IPCC第六次评估报告之冰冻圈变化解读     

钟歆玥  康世昌  郭万钦  吴晓东  陈金雷 《冰川冻土》2021,44(3):946-953

政府间气候变化专门委员会（IPCC）于2021年8月发布了第六次评估报告第一工作组报告《气候变化2021：自然科学基础》。该报告基于最新的观测和模拟研究,评估了冰冻圈变化的现状,并采用CMIP6模式对未来变化进行了预估。报告明确指出,近十多年来冰冻圈呈现加速萎缩状态：北极海冰面积显著减小、厚度减薄、冰量迅速减少;格陵兰冰盖、南极冰盖和全球山地冰川物质亏损加剧;多年冻土温度升高、活动层增厚,海底多年冻土范围减少;北半球积雪范围也在明显变小,但积雪量有较大空间差异。冰冻圈的快速萎缩加速海平面的上升。未来人类活动对冰冻圈萎缩的影响将愈加显著,从而导致北极海冰面积继续减少乃至消失,冰盖和冰川物质将持续亏损,多年冻土和积雪的范围继续缩减。报告也提出,目前冰冻圈研究仍存在观测资料稀缺、模型对各影响因素的敏感性参数和过程描述亟需提升、对吸光性杂质的变化机制认知不足等问题,从而影响了对冰冻圈变化预估的准确性,未来需要重点关注。  相似文献   

辽河西部凹陷曙北地区沙四段薄砂层成因类型及分布规律     

宋兵  王波  刘兴周  刘少治  陈希光  卢文忠 《地质与资源》2021,30(6):698-706

为了明确辽河西部凹陷曙北地区沙河街组四段薄砂层成因类型及分布规律,从岩心、测井响应和地震反射特征等方面总结了各类成因薄砂层的识别标志,并预测了各砂层组的砂体展布,探讨了砂体发育的控制因素,总结了沉积模式.研究结果表明,曙北地区沙四段为扇三角洲-湖泊的沉积体系,薄砂层发育水下分流河道、河口坝、低隆滩坝、沿岸浅滩4种成因类型,其中以水下分流河道和低隆滩坝为主.古地貌、古物源和古水深控制了各类砂体的展布.以曙光和兴隆台古潜山一线为界,南部为扇三角洲体系沉积区,主要发育前缘水下分流河道和河口坝;北部（包括低隆区）为无明显水流注入的半封闭湖湾区,主要发育低隆滩坝砂体和灰/云坪,在西侧沿岸局部地区还发育沿岸浅滩.储量区外大面积发育的低隆滩坝砂体,是下一步碎屑岩增储上产的潜在接替区域.  相似文献   

高时空分辨率三维风场在强对流天气临近预报中的融合应用研究   总被引：1，自引：0，他引：1       下载免费PDF全文

杨璐  陈敏  陈明轩  高峰  秦睿  宋林烨  程丛兰 《气象学报》2019,77(2):243-255

以业务应用为目标,开展高时、空分辨率三维风场在强对流天气临近预报中的融合应用研究。运用北京快速更新多尺度分析和预报系统集成子系统（RMAPS-IN,Rapid-refresh Multi-scale Analysis and Prediction System-Integration）,对雷达四维变分分析系统（VDRAS）30 min临近预报的高时、空分辨率三维风场作为数据源与自动气象站风场观测进行快速融合处理。结果表明,以VDRAS临近预报风场取代数值模式预报场作为融合初猜场后形成的分析结果对于风场有明显的改善:（1）长时间序列客观检验结果表明,地面10 m高风场U/V分量绝对误差分别为0.05和0.06 m/s。实时融合对未来预报的影响随着预报时效的延长,U/V分量的绝对误差不断增大。（2）对于11个强对流个例,地面10 m高风场风速均方根误差降低0.3 m/s,风向均方根误差降低13°;边界层三维风场,风速均方根误差降低0.8 m/s,风向均方根误差降低10°。平原站点融合以后风速、风向预报效果有较大改善,山区站点融合以后改善相对较小。（3）通过对2017年7月20日暴雨和7月7日雷暴大风个例的详细分析,发现融合基于雷达资料四维变分同化获得的高分辨率临近预报风场对各对流系统中的中尺度结构特征给出了更加细致准确的描述。   相似文献   

南海北部神狐海域细粒储层矿物组分对天然气水合物储集赋存的影响     

徐小蕾  白辰阳  苏丕波  马倩  张宇  梁金强 《地质论评》2023,69(6):2023060012-2023060012

为了探明矿物类型对于天然气水合物成藏的影响,笔者等利用南海北部神狐海域W07站位样品及其水合物饱和度数据,进行XRD全岩和黏土矿物测试分析、比表面积分析以及束缚水能力综合分析。结果表明,海床下110~127 m（即110~127 mbsf,meters below sea floor, 海床以下深度）为水合物储层段,海床下127~156 m为非水合物储层段。通过XRD分析可知,高石英及长石含量,低伊蒙混层含量的层段,比表面积与束缚水能力较低,说明其具有相对较好的孔渗条件,为水合物的运移与储集提供了良好的空间条件,因此形成水合物储层段;而在高伊蒙混层的层段中,比表面积较大,束缚水能力较强,其对甲烷气体及流体的吸附和束缚能力较强,对水合物成藏起到潜在的封隔作用,成为非储层段,储层与非储层段纵向叠置序列有利于优质水合物储层的形成。本次研究总结了矿物组分与优质水合物储层之间的关系,并揭示两者存在的潜在成因联系,以期丰富水合物富集成藏的基础理论,对未来南海北部天然气水合物的商业化开发提供支持。  相似文献   

Abiotic Methane Reservoirs in the Western Tianshan HP–UHP Metamorphic Belt,China          下载免费PDF全文

ZHANG Lijuan  ZHANG Lifei  LI Xiaowei  WANG Xiao 《《地质学报》英文版》2023,97(1):337-349

Natural gas, consisting primarily of methane(CH₄), has become a major source of clean energy in modern society in many parts of the globe. Recent experimental observations and discoveries of deep-sourced abiotic CH₄ in cold subduction zones indicate the important ability of cold subducted slabs to generate natural gas reservoirs. However, most CH₄ flux and reservoirs remain unknown and their potential is overlooked in global carbon flux estimations. Massive abiot...  相似文献   

鄂尔多斯盆地奥陶系马家沟组四段构造- 岩相古地理新认识及勘探意义     

于洲  王维斌  魏柳斌  李辉  吴东旭  乔占峰  吴兴宁  鲁慧丽  刘雨昕  胡文中 《地质学报》2023,97(8):2645-2658

米探1井取得天然气勘探突破表明鄂尔多斯盆地奥陶系马家沟组四段具有巨大勘探潜力,然而,对盆地奥陶纪马四期古构造格局和岩相古地理研究还存在争议,制约了下步天然气勘探进程。为此,基于地震、野外露头、钻井、岩芯、微观薄片和测井等基础资料,对马家沟组四段构造- 岩相古地理开展了系统研究,确定了盆地奥陶纪马四期古构造格局,并恢复出马家沟组四段岩相古地理,预测了有利勘探区。研究结果表明：① 鄂尔多斯盆地奥陶纪马四期发育“两陆三隆四坳”的古构造格局,其中两陆为伊盟古陆和阿拉善古陆,三隆分别为中央古隆起、中条古隆起和神木- 志丹低隆起,四坳为西南边缘坳陷、桃利庙坳陷、府谷坳陷和柳林坳陷;② 马四期为碳酸盐岩内缓坡和中缓坡沉积,其中内缓坡又发育白云岩坪、含云膏坪、微生物丘、灰泥丘、砂屑滩、丘滩间海和灰质潟湖等7类微相;③ 古构造格局控制马家沟组四段沉积分异,微生物丘、灰泥丘和砂屑滩等3类有利储集相主要沿中央古隆起和神木- 志丹低隆起等古地貌高部位分布。因此认为,神木—靖边地区是有利储层发育区,且处于岩性相变带,生储盖配置关系好,具有良好的成藏条件,是天然气勘探的有利靶向区。  相似文献   

苯并（a）芘诱导下岩虫CYP基因的表达特征     

李婉娟  赵欢  Ba Fuyang  李绍娟  孙秀鹏  杨大佐  周一兵 《海洋学报(英文版)》2019,38(6):46-53

Rapid amplification of cDNA ends(RACE) and real-time polymerase chain reaction(RT-PCR) were carried out to analyze the CYP4 gene expression in polychaete Marphysa sanguinea exposed to benzo[a]pyrene(BaP) in this study. The full length of MsCYP4 cDNA was 2 470 bp, and it encoded 512 amino acids. The deduced amino acid sequence showed 47% identity with CYP4 F from frog Xenopus tropicalis and shared high homology with other known CYP4 sequences. To analyse the role of CYP4 in protecting M. sanguinea from BaP exposure, three BaP groups were established: 0.5, 5 and 50 μg/L. Polychaetes were sampled after 3, 7 and 12 d. At 0.5 μg/L, the effect of BaP on MsCYP4 gene expression increased with time prolonged. MsCYP4 gene expression curve showed Ushaped trend with time in 5 and 50 μg/L BaP groups. Therefore, MsCYP4 gene may play an important role in maintaining the balance of cellular metabolism and protecting M. sanguinea from BaP toxicity.  相似文献   

Copper Isotopic Analysis in Geological and Biological Reference Materials by MC‐ICP‐MS     

Kaj Sullivan  Daniel Layton‐Matthews  Matthew Leybourne  James Kidder  Zoltn Mester  Lu Yang 《Geostandards and Geoanalytical Research》2020,44(2):349-362

The characterisation of relative copper isotope amount ratios (δ⁶⁵Cu) helps constrain a variety of geochemical processes occurring in the geosphere, biosphere and hydrosphere. The accurate and precise determination of δ⁶⁵Cu in matrix reference materials is crucial in the effort to validate measurement methods. With the goal of expanding the number and variety of available geological and biological materials, we have characterised the δ⁶⁵Cu values of ten reference materials by MC‐ICP‐MS using C‐SSBIN model for mass bias correction. SGR‐1b (Green River shale), DOLT‐5 (dogfish liver), DORM‐4 (fish protein), TORT‐3 (lobster hepatopancreas), MESS‐4 (marine sediment) and PACS‐3 (marine sediment) have for the first time been characterised for δ⁶⁵Cu. Additionally, four reference materials (with published δ⁶⁵Cu values) have been characterised: BHVO‐1 (Hawaiian basalt), BIR‐1 (Icelandic basalt), W‐2a (diabase) and Seronorm? Trace Elements Serum L‐1 (human serum). The reference materials measured in this study possess complex and varied matrices with copper mass fractions ranging from 1.2 µg g^?1 to 497 µg g^?1 and δ⁶⁵Cu values ranging from ?0.20‰ to 0.52‰ with a mean expanded uncertainty of ± 0.07‰ (U, k = 2), covering much of the natural copper isotope variability observed in the environment.  相似文献   

Application of a Bayesian model to infer the contribution of coalbed natural gas produced water to the Powder River,Wyoming and Montana          下载免费PDF全文

Jason M. Mailloux  Kiona Ogle  Carol D. Frost 《水文研究》2014,28(4):2361-2381

The Powder River Basin (PRB) of Wyoming and Montana contains significant coal and coal bed natural gas (CBNG) resources. CBNG extraction requires the production of large volumes of water, much of which is discharged into existing drainages. Compared to surface waters, the CBNG produced water is high in sodium relative to calcium and magnesium, elevating the sodium adsorption ratio (SAR). To mitigate the possible impact this produced water may have on the quality of surface water used for irrigation, the State of Montana passed water anti‐degradation legislation, which could affect CBNG production in Wyoming. In this study, we sought to determine the proportion of CBNG produced water discharged to tributaries that reaches the Powder River by implementing a four end‐member mixing model within a Bayesian statistical framework. The model accounts for the ⁸⁷Sr/⁸⁶Sr, δ¹³C_DIC, [Sr] and [DIC] of CBNG produced water and surface water interacting with the three primary lithologies exposed in the PRB. The model estimates the relative contribution of the end members to the river water, while incorporating uncertainty associated with measurement and process error. Model results confirm that both of the tributaries associated with high CBNG activity are mostly composed of CBNG produced water (70–100%). The model indicates that up to 50% of the Powder River is composed of CBNG produced water downstream from the CBNG tributaries, decreasing with distance by dilution from non‐CBNG impacted tributaries from the point sources to ~10–20% at the Montana border. This amount of CBNG produced water does not significantly affect the SAR or electrical conductivity of the Powder River in Montana. Copyright © 2013 John Wiley & Sons, Ltd.  相似文献